STEM Image Analysis Based on Deep Learning: Identification of Vacancy Defects and Polymorphs of MoS2

Kihyun Lee, Jinsub Park, Soyeon Choi, Yangjin Lee, Sol Lee, Joowon Jung, Jong Young Lee, Farman Ullah, Zeeshan Tahir, Yong Soo Kim, Gwan Hyoung Lee, Kwanpyo Kim

Research output: Contribution to journalArticlepeer-review

15 Citations (Scopus)

Abstract

Scanning transmission electron microscopy (STEM) is an indispensable tool for atomic-resolution structural analysis for a wide range of materials. The conventional analysis of STEM images is an extensive hands-on process, which limits efficient handling of high-throughput data. Here, we apply a fully convolutional network (FCN) for identification of important structural features of two-dimensional crystals. ResUNet, a type of FCN, is utilized in identifying sulfur vacancies and polymorph types of MoS2 from atomic resolution STEM images. Efficient models are achieved based on training with simulated images in the presence of different levels of noise, aberrations, and carbon contamination. The accuracy of the FCN models toward extensive experimental STEM images is comparable to that of careful hands-on analysis. Our work provides a guideline on best practices to train a deep learning model for STEM image analysis and demonstrates FCN's application for efficient processing of a large volume of STEM data.

Original languageEnglish
Pages (from-to)4677-4685
Number of pages9
JournalNano letters
Volume22
Issue number12
DOIs
Publication statusPublished - 2022 Jun 22

Bibliographical note

Publisher Copyright:
© 2022 The Authors. Published by American Chemical Society.

All Science Journal Classification (ASJC) codes

  • Bioengineering
  • General Chemistry
  • General Materials Science
  • Condensed Matter Physics
  • Mechanical Engineering

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