H2 and CO production over a stable Ni-MgO-Ce 0.8Zr0.2O2 catalyst from CO2 reforming of CH4

Won Jun Jang; Dae Woon Jeong; Jae Oh Shim; Hyun Seog Roh; In Hyuk Son; Seung Jae Lee

doi:10.1016/j.ijhydene.2013.01.196

H₂ and CO production over a stable Ni-MgO-Ce _0.8Zr_0.2O₂ catalyst from CO₂ reforming of CH₄

Won Jun Jang, Dae Woon Jeong, Jae Oh Shim, Hyun Seog Roh, In Hyuk Son, Seung Jae Lee

Division of Environmental Engineering

Research output: Contribution to journal › Article › peer-review

63 Citations (Scopus)

Abstract

Ni-Ce_0.8Zr_0.2O₂ and Ni-MgO-Ce _0.8Zr_0.2O₂ catalysts were investigated for H₂ production from CO₂ reforming of CH₄ reaction at a very high gas hourly space velocity of 480,000 h^-1. Ni-MgO-Ce_0.8Zr_0.2O₂ exhibited higher catalytic activity and stability (CH₄ conversion >95% at 800°C for 200 h). The outstanding catalytic performance is mainly due to the basic nature of MgO and an intimate interaction between Ni and MgO.

Original language	English
Pages (from-to)	4508-4512
Number of pages	5
Journal	International Journal of Hydrogen Energy
Volume	38
Issue number	11
DOIs	https://doi.org/10.1016/j.ijhydene.2013.01.196
Publication status	Published - 2013 Apr 15

Bibliographical note

Funding Information:
The authors gratefully acknowledge financial support from the Samsung Advanced Institute of Technology (SAIT), Samsung Electronics Co. Ltd. This Research was supported by a Basic Science Research Program through the National Research Foundation of Korea (NRF), funded by the Ministry of Education, Science and Technology ( 2010-0002521 ).

All Science Journal Classification (ASJC) codes

Renewable Energy, Sustainability and the Environment
Fuel Technology
Condensed Matter Physics
Energy Engineering and Power Technology

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

Access to Document

10.1016/j.ijhydene.2013.01.196

Cite this

@article{1722f8c8094d4d5d86cb76960221b628,

title = "H2 and CO production over a stable Ni-MgO-Ce 0.8Zr0.2O2 catalyst from CO2 reforming of CH4",

abstract = "Ni-Ce0.8Zr0.2O2 and Ni-MgO-Ce 0.8Zr0.2O2 catalysts were investigated for H2 production from CO2 reforming of CH4 reaction at a very high gas hourly space velocity of 480,000 h-1. Ni-MgO-Ce0.8Zr0.2O2 exhibited higher catalytic activity and stability (CH4 conversion >95% at 800°C for 200 h). The outstanding catalytic performance is mainly due to the basic nature of MgO and an intimate interaction between Ni and MgO.",

author = "Jang, {Won Jun} and Jeong, {Dae Woon} and Shim, {Jae Oh} and Roh, {Hyun Seog} and Son, {In Hyuk} and Lee, {Seung Jae}",

note = "Funding Information: The authors gratefully acknowledge financial support from the Samsung Advanced Institute of Technology (SAIT), Samsung Electronics Co. Ltd. This Research was supported by a Basic Science Research Program through the National Research Foundation of Korea (NRF), funded by the Ministry of Education, Science and Technology ( 2010-0002521 ).",

year = "2013",

month = apr,

day = "15",

doi = "10.1016/j.ijhydene.2013.01.196",

language = "English",

volume = "38",

pages = "4508--4512",

journal = "International Journal of Hydrogen Energy",

issn = "0360-3199",

publisher = "Elsevier Limited",

number = "11",

}

TY - JOUR

T1 - H2 and CO production over a stable Ni-MgO-Ce 0.8Zr0.2O2 catalyst from CO2 reforming of CH4

AU - Jang, Won Jun

AU - Jeong, Dae Woon

AU - Shim, Jae Oh

AU - Roh, Hyun Seog

AU - Son, In Hyuk

AU - Lee, Seung Jae

N1 - Funding Information: The authors gratefully acknowledge financial support from the Samsung Advanced Institute of Technology (SAIT), Samsung Electronics Co. Ltd. This Research was supported by a Basic Science Research Program through the National Research Foundation of Korea (NRF), funded by the Ministry of Education, Science and Technology ( 2010-0002521 ).

PY - 2013/4/15

Y1 - 2013/4/15

N2 - Ni-Ce0.8Zr0.2O2 and Ni-MgO-Ce 0.8Zr0.2O2 catalysts were investigated for H2 production from CO2 reforming of CH4 reaction at a very high gas hourly space velocity of 480,000 h-1. Ni-MgO-Ce0.8Zr0.2O2 exhibited higher catalytic activity and stability (CH4 conversion >95% at 800°C for 200 h). The outstanding catalytic performance is mainly due to the basic nature of MgO and an intimate interaction between Ni and MgO.

AB - Ni-Ce0.8Zr0.2O2 and Ni-MgO-Ce 0.8Zr0.2O2 catalysts were investigated for H2 production from CO2 reforming of CH4 reaction at a very high gas hourly space velocity of 480,000 h-1. Ni-MgO-Ce0.8Zr0.2O2 exhibited higher catalytic activity and stability (CH4 conversion >95% at 800°C for 200 h). The outstanding catalytic performance is mainly due to the basic nature of MgO and an intimate interaction between Ni and MgO.

UR - http://www.scopus.com/inward/record.url?scp=84875364554&partnerID=8YFLogxK

UR - http://www.scopus.com/inward/citedby.url?scp=84875364554&partnerID=8YFLogxK

U2 - 10.1016/j.ijhydene.2013.01.196

DO - 10.1016/j.ijhydene.2013.01.196

M3 - Article

AN - SCOPUS:84875364554

SN - 0360-3199

VL - 38

SP - 4508

EP - 4512

JO - International Journal of Hydrogen Energy

JF - International Journal of Hydrogen Energy

IS - 11

ER -