Fully Elastic Conductive Films from Viscoelastic Composites

Sunghwan Cho, Jun Hyuk Song, Minsik Kong, Sangbaie Shin, Young Tae Kim, Gyeongbae Park, Chan Gyung Park, Tae Joo Shin, Jaemin Myoung, Unyong Jeong

Research output: Contribution to journalArticlepeer-review

18 Citations (Scopus)


We investigated, for the first time, the conditions where a thermoplastic conductive composite can exhibit completely reversible stretchability at high elongational strains (= 1.8). We studied a composite of Au nanosheets and a polystyrene-block-polybutadiene-block-polystyrene block copolymer as an example. The composite had an outstandingly low sheet resistance (0.45 /sq). We found that when a thin thermoplastic composite film is placed on a relatively thicker chemically cross-linked elastomer film, it can follow the reversible elastic behavior of the bottom elastomer. Such elasticity comes from the restoration of the block copolymer microstructure. The strong adhesion of the thermoplastic polymer to the metallic fillers is advantageous in the fabrication of mechanically robust, highly conductive, stretchable electrodes. The chemical stability of the Au composite was used to fabricate high luminescence, stretchable electrochemiluminescence displays with a conventional top-bottom electrode setup and with a horizontal electrode setup.

Original languageEnglish
Pages (from-to)44096-44105
Number of pages10
JournalACS Applied Materials and Interfaces
Issue number50
Publication statusPublished - 2017 Dec 20

Bibliographical note

Publisher Copyright:
© 2017 American Chemical Society.

All Science Journal Classification (ASJC) codes

  • Materials Science(all)


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