Feasibility study of polyetherimide membrane for enrichment of carbon dioxide from synthetic biohydrogen mixture and subsequent utilization scenario using microalgae

Péter Bakonyi; Jakub Peter; Nándor Nemestóthy; David Malý; Gopalakrishnan Kumar; Stanislaw Koter; Sang Hyoun Kim; Wojciech Kujawski; Katalin Bélafi-Bakó; Zbynek Pientka

doi:10.1002/er.5732

Feasibility study of polyetherimide membrane for enrichment of carbon dioxide from synthetic biohydrogen mixture and subsequent utilization scenario using microalgae

Péter Bakonyi, Jakub Peter, Nándor Nemestóthy, David Malý, Gopalakrishnan Kumar, Stanislaw Koter, Sang Hyoun Kim, Wojciech Kujawski, Katalin Bélafi-Bakó, Zbynek Pientka

Department of Civil and Environmental Engineering

Research output: Contribution to journal › Article › peer-review

Abstract

In this work, the potential of utilizing a polyetherimide (PEI) hollow-fiber membrane to separate synthetic biohydrogen mixture (H₂/CO₂) was studied. From the gas separation experiments, where the effects of feed to permeate pressure ratio (P_feed/P_permeate) and stage-cut as key factors were evaluated, it was found that the PEI membrane had the capacity to purify either H₂ or CO₂. It turned out that different separation settings should be chosen in accordance with the actual technological purpose, defined either as the enrichment of H₂ or CO₂. The highest H₂ concentration (66.4 vol%) in the permeate was achieved at P_feed/P_permeate of 4.62 and stage-cut of 0.47, while the peak CO₂ concentration (79.2 vol%) in the retentate was obtained by applying P_feed/P_permeate of 4.55 and stage-cut of 0.65. The assessment and discussion of results indicated the possible utilization of the CO₂-rich fraction (produced by the PEI membrane) for the biological sequestration using microalgae. To our knowledge, PEI membranes have not yet been tested in such a concept and thus, the results and experiences can mean a new contribution to the literature.

Original language	English
Pages (from-to)	8327-8334
Number of pages	8
Journal	International Journal of Energy Research
Volume	45
Issue number	6
DOIs	https://doi.org/10.1002/er.5732
Publication status	Published - 2021 May

Bibliographical note

Funding Information:
Ministerstvo Školství, Mládeže a Tělovýchovy, Grant/Award Number: MSMT‐20364/2017‐3/5; Narodowe Centrum Badań i Rozwoju, Grant/Award Number: DZP/V4‐Korea‐1/190/2018; National Research Foundation of Korea, Grant/Award Number: 2017K1A3A1A67015923; Nemzeti Kutatási Fejlesztési és Innovációs Hivatal, Grant/Award Number: NN 126995 Funding information

Funding Information:
The authors would like to acknowledge their respective funding schemes for supporting this work: National Research, Development, and Innovation Office (NKFIH, Hungary) (grant number NN 126995); International Research & Development Program of the National Research Foundation of Korea (NRF) funded by the Ministry of Science & ICT (grant number: 2017K1A3A1A67015923); National Centre for Research and Development, Poland (DZP/V4‐Korea‐1/190/2018); Czech Ministry of Education, Youth and Sport (project 8F17005, contract no. MSMT‐20364/2017‐3/5).

Funding Information:
The authors would like to acknowledge their respective funding schemes for supporting this work: National Research, Development, and Innovation Office (NKFIH, Hungary) (grant number NN 126995); International Research & Development Program of the National Research Foundation of Korea (NRF) funded by the Ministry of Science & ICT (grant number: 2017K1A3A1A67015923); National Centre for Research and Development, Poland (DZP/V4-Korea-1/190/2018); Czech Ministry of Education, Youth and Sport (project 8F17005, contract no. MSMT-20364/2017-3/5).

Publisher Copyright:
© 2020 The Authors. International Journal of Energy Research published by John Wiley & Sons Ltd.

All Science Journal Classification (ASJC) codes

Renewable Energy, Sustainability and the Environment
Nuclear Energy and Engineering
Fuel Technology
Energy Engineering and Power Technology

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

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10.1002/er.5732

Cite this

Bakonyi, P., Peter, J., Nemestóthy, N., Malý, D., Kumar, G., Koter, S., Kim, S. H., Kujawski, W., Bélafi-Bakó, K., & Pientka, Z. (2021). Feasibility study of polyetherimide membrane for enrichment of carbon dioxide from synthetic biohydrogen mixture and subsequent utilization scenario using microalgae. International Journal of Energy Research, 45(6), 8327-8334. https://doi.org/10.1002/er.5732

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title = "Feasibility study of polyetherimide membrane for enrichment of carbon dioxide from synthetic biohydrogen mixture and subsequent utilization scenario using microalgae",

abstract = "In this work, the potential of utilizing a polyetherimide (PEI) hollow-fiber membrane to separate synthetic biohydrogen mixture (H2/CO2) was studied. From the gas separation experiments, where the effects of feed to permeate pressure ratio (Pfeed/Ppermeate) and stage-cut as key factors were evaluated, it was found that the PEI membrane had the capacity to purify either H2 or CO2. It turned out that different separation settings should be chosen in accordance with the actual technological purpose, defined either as the enrichment of H2 or CO2. The highest H2 concentration (66.4 vol%) in the permeate was achieved at Pfeed/Ppermeate of 4.62 and stage-cut of 0.47, while the peak CO2 concentration (79.2 vol%) in the retentate was obtained by applying Pfeed/Ppermeate of 4.55 and stage-cut of 0.65. The assessment and discussion of results indicated the possible utilization of the CO2-rich fraction (produced by the PEI membrane) for the biological sequestration using microalgae. To our knowledge, PEI membranes have not yet been tested in such a concept and thus, the results and experiences can mean a new contribution to the literature.",

author = "P{\'e}ter Bakonyi and Jakub Peter and N{\'a}ndor Nemest{\'o}thy and David Mal{\'y} and Gopalakrishnan Kumar and Stanislaw Koter and Kim, {Sang Hyoun} and Wojciech Kujawski and Katalin B{\'e}lafi-Bak{\'o} and Zbynek Pientka",

note = "Funding Information: Ministerstvo {\v S}kolstv{\'i}, Ml{\'a}de{\v z}e a T{\v e}lov{\'y}chovy, Grant/Award Number: MSMT‐20364/2017‐3/5; Narodowe Centrum Bada{\'n} i Rozwoju, Grant/Award Number: DZP/V4‐Korea‐1/190/2018; National Research Foundation of Korea, Grant/Award Number: 2017K1A3A1A67015923; Nemzeti Kutat{\'a}si Fejleszt{\'e}si {\'e}s Innov{\'a}ci{\'o}s Hivatal, Grant/Award Number: NN 126995 Funding information Funding Information: The authors would like to acknowledge their respective funding schemes for supporting this work: National Research, Development, and Innovation Office (NKFIH, Hungary) (grant number NN 126995); International Research & Development Program of the National Research Foundation of Korea (NRF) funded by the Ministry of Science & ICT (grant number: 2017K1A3A1A67015923); National Centre for Research and Development, Poland (DZP/V4‐Korea‐1/190/2018); Czech Ministry of Education, Youth and Sport (project 8F17005, contract no. MSMT‐20364/2017‐3/5). Funding Information: The authors would like to acknowledge their respective funding schemes for supporting this work: National Research, Development, and Innovation Office (NKFIH, Hungary) (grant number NN 126995); International Research & Development Program of the National Research Foundation of Korea (NRF) funded by the Ministry of Science & ICT (grant number: 2017K1A3A1A67015923); National Centre for Research and Development, Poland (DZP/V4-Korea-1/190/2018); Czech Ministry of Education, Youth and Sport (project 8F17005, contract no. MSMT-20364/2017-3/5). Publisher Copyright: {\textcopyright} 2020 The Authors. International Journal of Energy Research published by John Wiley & Sons Ltd.",

year = "2021",

month = may,

doi = "10.1002/er.5732",

language = "English",

volume = "45",

pages = "8327--8334",

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Bakonyi, P, Peter, J, Nemestóthy, N, Malý, D, Kumar, G, Koter, S, Kim, SH, Kujawski, W, Bélafi-Bakó, K & Pientka, Z 2021, 'Feasibility study of polyetherimide membrane for enrichment of carbon dioxide from synthetic biohydrogen mixture and subsequent utilization scenario using microalgae', International Journal of Energy Research, vol. 45, no. 6, pp. 8327-8334. https://doi.org/10.1002/er.5732

Feasibility study of polyetherimide membrane for enrichment of carbon dioxide from synthetic biohydrogen mixture and subsequent utilization scenario using microalgae. / Bakonyi, Péter; Peter, Jakub; Nemestóthy, Nándor et al.
In: International Journal of Energy Research, Vol. 45, No. 6, 05.2021, p. 8327-8334.

Research output: Contribution to journal › Article › peer-review

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AU - Peter, Jakub

AU - Nemestóthy, Nándor

AU - Malý, David

AU - Kumar, Gopalakrishnan

AU - Koter, Stanislaw

AU - Kim, Sang Hyoun

AU - Kujawski, Wojciech

AU - Bélafi-Bakó, Katalin

AU - Pientka, Zbynek

N1 - Funding Information: Ministerstvo Školství, Mládeže a Tělovýchovy, Grant/Award Number: MSMT‐20364/2017‐3/5; Narodowe Centrum Badań i Rozwoju, Grant/Award Number: DZP/V4‐Korea‐1/190/2018; National Research Foundation of Korea, Grant/Award Number: 2017K1A3A1A67015923; Nemzeti Kutatási Fejlesztési és Innovációs Hivatal, Grant/Award Number: NN 126995 Funding information Funding Information: The authors would like to acknowledge their respective funding schemes for supporting this work: National Research, Development, and Innovation Office (NKFIH, Hungary) (grant number NN 126995); International Research & Development Program of the National Research Foundation of Korea (NRF) funded by the Ministry of Science & ICT (grant number: 2017K1A3A1A67015923); National Centre for Research and Development, Poland (DZP/V4‐Korea‐1/190/2018); Czech Ministry of Education, Youth and Sport (project 8F17005, contract no. MSMT‐20364/2017‐3/5). Funding Information: The authors would like to acknowledge their respective funding schemes for supporting this work: National Research, Development, and Innovation Office (NKFIH, Hungary) (grant number NN 126995); International Research & Development Program of the National Research Foundation of Korea (NRF) funded by the Ministry of Science & ICT (grant number: 2017K1A3A1A67015923); National Centre for Research and Development, Poland (DZP/V4-Korea-1/190/2018); Czech Ministry of Education, Youth and Sport (project 8F17005, contract no. MSMT-20364/2017-3/5). Publisher Copyright: © 2020 The Authors. International Journal of Energy Research published by John Wiley & Sons Ltd.

PY - 2021/5

Y1 - 2021/5

N2 - In this work, the potential of utilizing a polyetherimide (PEI) hollow-fiber membrane to separate synthetic biohydrogen mixture (H2/CO2) was studied. From the gas separation experiments, where the effects of feed to permeate pressure ratio (Pfeed/Ppermeate) and stage-cut as key factors were evaluated, it was found that the PEI membrane had the capacity to purify either H2 or CO2. It turned out that different separation settings should be chosen in accordance with the actual technological purpose, defined either as the enrichment of H2 or CO2. The highest H2 concentration (66.4 vol%) in the permeate was achieved at Pfeed/Ppermeate of 4.62 and stage-cut of 0.47, while the peak CO2 concentration (79.2 vol%) in the retentate was obtained by applying Pfeed/Ppermeate of 4.55 and stage-cut of 0.65. The assessment and discussion of results indicated the possible utilization of the CO2-rich fraction (produced by the PEI membrane) for the biological sequestration using microalgae. To our knowledge, PEI membranes have not yet been tested in such a concept and thus, the results and experiences can mean a new contribution to the literature.

AB - In this work, the potential of utilizing a polyetherimide (PEI) hollow-fiber membrane to separate synthetic biohydrogen mixture (H2/CO2) was studied. From the gas separation experiments, where the effects of feed to permeate pressure ratio (Pfeed/Ppermeate) and stage-cut as key factors were evaluated, it was found that the PEI membrane had the capacity to purify either H2 or CO2. It turned out that different separation settings should be chosen in accordance with the actual technological purpose, defined either as the enrichment of H2 or CO2. The highest H2 concentration (66.4 vol%) in the permeate was achieved at Pfeed/Ppermeate of 4.62 and stage-cut of 0.47, while the peak CO2 concentration (79.2 vol%) in the retentate was obtained by applying Pfeed/Ppermeate of 4.55 and stage-cut of 0.65. The assessment and discussion of results indicated the possible utilization of the CO2-rich fraction (produced by the PEI membrane) for the biological sequestration using microalgae. To our knowledge, PEI membranes have not yet been tested in such a concept and thus, the results and experiences can mean a new contribution to the literature.

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Feasibility study of polyetherimide membrane for enrichment of carbon dioxide from synthetic biohydrogen mixture and subsequent utilization scenario using microalgae

Abstract

Bibliographical note

All Science Journal Classification (ASJC) codes

UN SDGs

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