Composition Control of Plasmon-Phonon Interaction Using Topological Quantum-Phase Transition in Photoexcited (Bi1-xInx)2Se3

Sangwan Sim, Jun Park, Nikesh Koirala, Seungmin Lee, Matthew Brahlek, Jisoo Moon, Maryam Salehi, Jaeseok Kim, Soonyoung Cha, Ji Ho Sung, Moon Ho Jo, Seongshik Oh, Hyunyong Choi

Research output: Contribution to journalArticlepeer-review

10 Citations (Scopus)


Plasmonics is a technology aiming at light modulation via collective charge oscillations. Topological insulators, where Dirac-like metallic surfaces coexist with normal insulating bulk, have recently attracted great attention in plasmonics due to their topology-originated outstanding properties. Here, we introduce a new methodology for controlling the interaction of a plasmon with a phonon in topological insulators, which is a key for utilizing the unique spectral profiles for photonic applications. By using both static and ultrafast terahertz spectroscopy, we show that the interaction can be tuned by controlling the chemical composition of (Bi1-xInx)2Se3 microribbon arrays. The topological quantum-phase transition induced by varying the composition drives a dramatic change in the strength of the plasmon-phonon interaction. This was possible due to the availability of manipulating the spatial overlap between topological surface plasmonic states and underlying bulk phonons. Especially, we control the laser-induced ultrafast evolution of the transient spectral peaks arising from the plasmon-phonon interaction by varying the spatial overlap across the topological phase transition. This study may provide a new platform for realizing topological insulator-based ultrafast plasmonic devices.

Original languageEnglish
Pages (from-to)1426-1431
Number of pages6
JournalACS Photonics
Issue number8
Publication statusPublished - 2016 Aug 17

Bibliographical note

Funding Information:
S.S., J.P., S.C., J.K., and H.C. were supported by the National Research Foundation of Korea (NRF) through the government of Korea (MSIP) (Grant Nos. NRF-2015R1A2A1A10052520, NRF-2016R1A4A1012929), Global Frontier Program (2014M3A6B3063709), the Yonsei University Yonsei-SNU Collaborative Research Fund of 2014, and the Yonsei University Future-Leading Research Initiative of 2014.

Publisher Copyright:
© 2016 American Chemical Society.

All Science Journal Classification (ASJC) codes

  • Electronic, Optical and Magnetic Materials
  • Biotechnology
  • Atomic and Molecular Physics, and Optics
  • Electrical and Electronic Engineering


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