An Ångström-level: D -spacing controlling synthetic route for MoS2 towards stable intercalation of sodium ions

Kan Zhang; Ping Li; Shiying Guo; Jong Yeob Jeong; Bingjun Jin; Xiaoming Li; Shengli Zhang; Haibo Zeng; Jong Hyeok Park

doi:10.1039/c8ta09066a

An Ångström-level: D -spacing controlling synthetic route for MoS₂ towards stable intercalation of sodium ions

Kan Zhang, Ping Li, Shiying Guo, Jong Yeob Jeong, Bingjun Jin, Xiaoming Li, Shengli Zhang, Haibo Zeng, Jong Hyeok Park

Department of Chemical and Biomolecular Engineering

Research output: Contribution to journal › Article › peer-review

24 Citations (Scopus)

Abstract

In this paper, we precisely controlled the d-spacing of vertically aligned MoS₂ arrays ranging from 6.2 to 10 Å via heating-controlled deintercalation of NH₄ ⁺ ions. The finely controllable interlayer nanoarchitecture resulted in an optimal d-spacing of 7.3 Å, which on nitrogenous reduced graphene oxide (N-RGO) delivered a reversible capacity of 295 mA h g^-1 after 2000 cycles at 1 A g^-1 for Na⁺ intercalation.

Original language	English
Pages (from-to)	22513-22518
Number of pages	6
Journal	Journal of Materials Chemistry A
Volume	6
Issue number	45
DOIs	https://doi.org/10.1039/c8ta09066a
Publication status	Published - 2018

Bibliographical note

Funding Information:
This work was supported by the NRF Korea (NRF-2016R1A2A1A05005216 and NRF-2017M3A7B4041987), NSFC (5151101197, 61725402, 51802157), the Fundamental Research Funds for the Central Universities (No. 30917011202, 30915012205, 30916015106 and 30918011106), the Natural Science Foundation of Jiangsu Province of China, No. BK20180493 and PAPD of Jiangsu Higher Education Institutions.

Publisher Copyright:
© The Royal Society of Chemistry.

All Science Journal Classification (ASJC) codes

Chemistry(all)
Renewable Energy, Sustainability and the Environment
Materials Science(all)

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

Access to Document

10.1039/c8ta09066a

Cite this

@article{294d36fed903416e9c9860acf470a760,

title = "An {\AA}ngstr{\"o}m-level: D -spacing controlling synthetic route for MoS2 towards stable intercalation of sodium ions",

abstract = "In this paper, we precisely controlled the d-spacing of vertically aligned MoS2 arrays ranging from 6.2 to 10 {\AA} via heating-controlled deintercalation of NH4 + ions. The finely controllable interlayer nanoarchitecture resulted in an optimal d-spacing of 7.3 {\AA}, which on nitrogenous reduced graphene oxide (N-RGO) delivered a reversible capacity of 295 mA h g-1 after 2000 cycles at 1 A g-1 for Na+ intercalation.",

author = "Kan Zhang and Ping Li and Shiying Guo and Jeong, {Jong Yeob} and Bingjun Jin and Xiaoming Li and Shengli Zhang and Haibo Zeng and Park, {Jong Hyeok}",

note = "Funding Information: This work was supported by the NRF Korea (NRF-2016R1A2A1A05005216 and NRF-2017M3A7B4041987), NSFC (5151101197, 61725402, 51802157), the Fundamental Research Funds for the Central Universities (No. 30917011202, 30915012205, 30916015106 and 30918011106), the Natural Science Foundation of Jiangsu Province of China, No. BK20180493 and PAPD of Jiangsu Higher Education Institutions. Publisher Copyright: {\textcopyright} The Royal Society of Chemistry.",

year = "2018",

doi = "10.1039/c8ta09066a",

language = "English",

volume = "6",

pages = "22513--22518",

journal = "Journal of Materials Chemistry A",

issn = "2050-7488",

publisher = "Royal Society of Chemistry",

number = "45",

}

TY - JOUR

T1 - An Ångström-level

T2 - D -spacing controlling synthetic route for MoS2 towards stable intercalation of sodium ions

AU - Zhang, Kan

AU - Li, Ping

AU - Guo, Shiying

AU - Jeong, Jong Yeob

AU - Jin, Bingjun

AU - Li, Xiaoming

AU - Zhang, Shengli

AU - Zeng, Haibo

AU - Park, Jong Hyeok

N1 - Funding Information: This work was supported by the NRF Korea (NRF-2016R1A2A1A05005216 and NRF-2017M3A7B4041987), NSFC (5151101197, 61725402, 51802157), the Fundamental Research Funds for the Central Universities (No. 30917011202, 30915012205, 30916015106 and 30918011106), the Natural Science Foundation of Jiangsu Province of China, No. BK20180493 and PAPD of Jiangsu Higher Education Institutions. Publisher Copyright: © The Royal Society of Chemistry.

PY - 2018

Y1 - 2018

N2 - In this paper, we precisely controlled the d-spacing of vertically aligned MoS2 arrays ranging from 6.2 to 10 Å via heating-controlled deintercalation of NH4 + ions. The finely controllable interlayer nanoarchitecture resulted in an optimal d-spacing of 7.3 Å, which on nitrogenous reduced graphene oxide (N-RGO) delivered a reversible capacity of 295 mA h g-1 after 2000 cycles at 1 A g-1 for Na+ intercalation.

AB - In this paper, we precisely controlled the d-spacing of vertically aligned MoS2 arrays ranging from 6.2 to 10 Å via heating-controlled deintercalation of NH4 + ions. The finely controllable interlayer nanoarchitecture resulted in an optimal d-spacing of 7.3 Å, which on nitrogenous reduced graphene oxide (N-RGO) delivered a reversible capacity of 295 mA h g-1 after 2000 cycles at 1 A g-1 for Na+ intercalation.

UR - http://www.scopus.com/inward/record.url?scp=85057006559&partnerID=8YFLogxK

UR - http://www.scopus.com/inward/citedby.url?scp=85057006559&partnerID=8YFLogxK

U2 - 10.1039/c8ta09066a

DO - 10.1039/c8ta09066a

M3 - Article

AN - SCOPUS:85057006559

SN - 2050-7488

VL - 6

SP - 22513

EP - 22518

JO - Journal of Materials Chemistry A

JF - Journal of Materials Chemistry A

IS - 45

ER -